DIELECTRIC PROPERTIES OF GLASS CERAMIC COMPOSITES FABRICATED VIA MICROWAVE TECHNIQUE

Authors

  • Somjit Lapnonkawow Department of Materials Science and Engineering, Faculty of Engineering and Industrial Technology, Silpakorn University, Nakhon Pathom, 73000, Thailand.
  • Sarawut Phupaichitkun Department of Materials Science and Engineering, Faculty of Engineering and Industrial Technology, Silpakorn University, Nakhon Pathom, 73000, Thailand.
  • Natthapong Wongdamnern Faculty of Science and Technology, Rajamangala University of Technology Suvarnabhumi, Nonthaburi, 11000, Thailand.
  • Thanapong Sareein Division of Industrial Materials Science, Faculty of Science and Technology, Rajamangala University of Technology, Phra Nakhon, 10800, Thailand.
  • Ekarat Meechoowas Department of Science Service, Ministry of Higher Education, Science, Research and Innovation (MHESI), Bangkok, 10400, Thailand.
  • Rattikarn Khankrua Department of Materials Engineering, Faculty of Engineering, Rajamangala University of Technology Rattanakosin, Salaya, Phutthamonthon, Nakhon Pathom, 73170, Thailand.
  • Narit Triamnak Department of Materials Science and Engineering, Faculty of Engineering and Industrial Technology, Silpakorn University, Nakhon Pathom, 73000, Thailand.

DOI:

https://doi.org/10.55766/sujst9383

Keywords:

Dielectric, Glass Ceramics, Microwave, Sustainable Energy, Titanium Dioxide

Abstract

The investigations and enhancement of dielectric ceramics have been studied for decades in order to improve their performance of sustainable management in energy. To increase dielectric constant, dielectric breakdown strength and to decrease dielectric loss have been generally focused. In this study, Ti0.98(Ni0.01, Nb0.01)O2, using as ceramics phase, and borosilicate glass powder were fabricated to glass ceramic composites with different concentration via microwave heating technique. X-ray diffraction technique and Raman spectroscopy revealed the crystalline phase existence in the glass ceramic composites. The results were also confirmed by Scanning Electron Microscope. Moreover, as the content of ceramic phase increased it was found that the dielectric constant increased and dielectric loss decreased.

References

Abdel Maksoud, M.I.A., Fahim, R.A., Shalan, A.E., Abd Elkodous, M., Olojede, S.O., Osman, A.I., Farrell, C., Al-Muhtaseb, A.H., Awed, A.S., Ashour, A.H., and Rooney, D.W. (2021). Advanced materials and technologies for supercapacitors used in energy conversion and storage: A review. Environmental Chemistry Letters, 19(1):375-439. https://doi.org/10.1007/s10311-020-01075-w

Buscaglia, M.T., Viviani, M., Buscaglia, V., Mitoseriu, L., Testino, A., and Nanni, P., Zhao, Z., Nygren, M., Harnagea, C., Piazza, D., and Galassi, C. (2006). High dielectric constant and frozen macroscopic polarization in dense nanocrystalline BaTiO3 ceramics. Physical Review B, 73(6):064114. DOI: 10.1103/PhysRevB.73.064114

Charoonsuk, T., Muanghlua, R., Sriphan, S., Pongampai, S., and Vittayakorn, N. (2021). Utilization of commodity thermoplastic polyethylene (PE) by enhanced sensing performance with liquid phase electrolyte for a flexible and transparent triboelectric tactile sensor. Sustainable Materials and Technologies, 27:e00239https://doi.org/10.1016/j.susmat.2020.e00239

Cheng, X., Li, Z., and Wu, J. (2015). Colossal permittivity in ceramics of TiO2 Co-doped with niobium and trivalent cation. Journal of Materials Chemistry A, 3(11):5805-5810. https://doi.org/10.1039/C5TA00141B

Chung, S.-Y., Kim, I.-D., and Kang, S.-J.L. (2004). Strong nonlinear current-voltage behaviour in perovskite-derivative calcium copper titanate. Nature Materials, 3(11):774-778. https://doi.org/10.1038/nmat1238

Dong, W., Hu, W., Frankcombe, T.J., Chen, D., Zhou, C., Fu, Z., Cândido, L., Hai, G., Chen, H., Li, Y., Withersa, R.L., and Liu, Y. (2017). Colossal permittivity with ultralow dielectric loss in In + Ta co-doped rutile TiO2. Journal of Materials Chemistry A, 5(11):5436-5441. https://doi.org/10.1039/C6TA08337D

Guo, B., Liu, P., Cui, X., and Song,Y. (2018). Colossal permittivity and dielectric relaxations in Tl + Nb co-doped TiO2 ceramics. Ceramics International, 44(11):12137 https://doi.org/10.1016/j.ceramint.2018.03.255

Kara, A. and Stevens, R. (2002). Interactions between an ABS type leadless glaze and a biscuit fired bone china body during glost firing. Part I: preparation of experimental phases. Journal of the European Ceramic Society, 22(7):1095-1102https://doi.org/10.1016/S0955-2219(01)00419-8

Prasatkhetragarn, A., Sareein, T., Triamnak, N., and Yimnirun, R. (2022). Dielectric and ferroelectric properties of modified-BaTiO3 lead-free ceramics prepared by solid solution method. Ferroelectrics, 586(1):224-241. https://doi.org/10.1080/00150193.2021.2014274

Pulphol, P., Pongampai, S., Charoonsuk, T., Vittayakorn, W., Muanghua, R., and Vittayakorn, N. (2022). Intrinsic enhancement of permittivity with ultralow dielectric loss in donor-acceptor co-doped rutile TiO2 ceramics. Integrated Ferroelectrics, 223(1):152-161. https://doi.org/10.1080/10584587.2021.1964294

Raengthon, N., Sebastian, T., Cumming, D., Reaney, I.M., and Cann, D.P. (2012). BaTiO3-Bi(Zn1/2Ti1/2)O3-BiScO3 ceramics for high-temperature capacitor applications. Journal of the American Ceramic Society, 95:3554-3561. https://doi.org/10.1111/j.1551-2916.2012.05340.x

Song, Y., Wang, X., Sui, Y., Liu, Z., Zhang, Y., Zhan, H., Song, B., Liu, Z., Lv, Z., Tao, L.,and Tang, J. (2016). Origin of colossal dielectric permittivity of rutile Ti0.9In0.05Nb0.05O2: Single crystal and polycrystalline, Sci. Rep. 6 (1), 21478 https://doi.org/10.1038/srep21478

Sriphan, S., Charoonsuk, T., Maluangnont, T., Vittayakorn, N. (2019). High-performance hybridized composited-based piezoelectric and triboelectric nanogenerators based on BaTiO3/PDMS composite film modified with Ti0.8O2 nanosheets and silver nanopowders cofillers. ACS Applied Energy Materials, 2(5):3840-3850. https://doi.org/10.1021/acsaem.9b00513

Triamnak, N., Brennecka, G.L., Brown-Shaklee, H.J., Rodriguez, M.A., and Cann, D.P. (2014). Phase formation of

BaTiO3-Bi(Zn1/2Ti1/2)O3 perovskite ceramics. Journal of the Ceramic Society of Japan, 122(1424):260-266 https://doi.org/10.2109/jcersj2.122.260

Triamnak, N., Suttiruengwong, S., Vittayakorn, N., Girdthep, S., and Khankrua, R. (2023). The Properties investigations of PLA/TiO2 and PLA/Doped-TiO2 composites films. Polymer-Plastics Technology and Materials, 62(12):1576-1586. https://doi.org/10.1080/25740881.2023.2222818

Triamnak, N., Wongdamnern, N., Sareein, T., Ngamjarurojana, A., and Yimnirun, R. (2022). Lowering Synthesis Temperature of BaTiO3-Bi(Zn0.5Zr0.5)O3 Ceramics by Salt Flux Assistance and Dielectric Properties Investigations. Integrated Ferroelectrics, 223(1):162-172. https://doi.org/10.1080/10584587.2021.1964295

Triamnak, N., Yimnirun, R., Pokorny, J., and Cann, D.P. (2013). Relaxor Characteristics of the Phase Transformation in (1−x)BaTiO3–xBi(Zn1/2Ti1/2)O3 Perovskite Ceramics. J. Am. Ceram. Soc., 96:3176-3182 https://doi.org/10.1111/jace.12495

Wang, Z., Yu, L., Fan, S., and Tan, X. (2013). Giant dielectric permittivity in Li and Nb doped NiO. Advanced Science Letters, 19(6):1763-1765. https://doi.org/10.1166/asl.2013.4522

Wei, X., Jie, W., Yang, Z., Zheng, F., Zeng, H., Liue, Y., and Hao, J. (2015). Colossal permittivity properties of Zn, Nb co-doped TiO2 with different phase structures. Journal of Materials Chemistry C, 3(42):11005-11010. https://doi.org/10.1039/C5TC02578H

Wu, J., Nan, C.-W., Lin, Y., and Deng, Y. (2002). Giant dielectric permittivity observed in Li and Ti doped NiO, Physical Review Letters, 89(21):217601. https://doi.org/10.1103/PhysRevLett.89.217601

Yao, Z., Song, Z., Hao, H., Yu, Z., Cao, M., Zhang, S., Lanagan, M.T., and Liu, H. (2017). Homogeneous/inhomogeneous-structured dielectrics and their energy-storage performances. Advanced Materials, 29(20):1601727. https://doi.org/10.1002/adma.201601727

Downloads

Published

2025-04-17

How to Cite

Lapnonkawow, S., Phupaichitkun, S., Wongdamnern, N., Sareein, T., Meechoowas, E., Khankrua, R., & Triamnak, N. (2025). DIELECTRIC PROPERTIES OF GLASS CERAMIC COMPOSITES FABRICATED VIA MICROWAVE TECHNIQUE. Suranaree Journal of Science and Technology, 32(1), 030287(1–7). https://doi.org/10.55766/sujst9383

Issue

Vol. 32 No. 1 (2025): January - February

Section

Research Article

Categories